[gmx-users] gold-S simulation

francesco oteri francesco.oteri at gmail.com
Sun Dec 16 04:34:20 CET 2012


Hi fatemeh,
I am looking for prameters like yours, where have you took the parameters
for gold and gold-aminoacid inteaction?

Francesco


2012/12/16 Peter C. Lai <pcl at uab.edu>

> Where is the .itp file for the system?
>
> On 2012-12-15 01:40:27PM -0800, fatemeh ramezani wrote:
> > hi
> >
> >
> > I'm simulating gold atom interaction with  aminoacidcys. I have made
> gold-cys.pdb by hyperchem software:
> >
> > HETATM    1  N   CYS     1       0.000   1.335   0.000
> > HETATM    2  CA  CYS     1      -0.683   1.818  -1.183
> > HETATM    3  C   CYS     1      -0.705   3.339  -1.221
> > HETATM    4  O   CYS     1      -0.184   3.993  -0.319
> > HETATM    5  CB  CYS     1      -2.127   1.330  -1.221
> > HETATM    6  SG  CYS     1      -3.106   1.859  -2.649
> > HETATM    8 AU   AU      8      -2.833   0.428  -1.793
> > HETATM    9 AU   AU      9      -2.647   0.381  -2.869
> > HETATM   10 AU   AU     10      -1.691   1.360  -3.093
> > HETATM   11 AU   AU     11      -0.647   2.706  -2.135
> > HETATM   12 AU   AU     12      -2.742   0.834  -0.456
> > HETATM   13 AU   AU     13      -1.691   2.061  -0.043
> > HETATM   14 AU   AU     14      -0.783   3.136   0.376
> > HETATM   15 AU   AU     15       0.095   3.750  -1.068
> > HETATM   16 AU   AU     16      -2.929   2.480  -2.204
> > HETATM   17 AU   AU     17      -3.285   1.594  -3.328
> > HETATM   18 AU   AU     18      -2.544   2.593  -3.763
> > HETATM   19 AU   AU     19      -1.951   1.260  -2.303
> > CONECT    1    2
> > CONECT    0    1
> > CONECT    2    1    3    5
> > CONECT    0    2
> > CONECT    3    2    4
> > CONECT    4    3
> > CONECT    5    2    6
> > CONECT    0    5
> > CONECT    0    5
> > CONECT    6    5
> > CONECT    0    6
> > CONECT    0    6
> > CONECT    0    6
> > END
> >
> >
> >
> > I started simulation by this pdb file. I'm using OPLSAA force field and
> also I added gold parameter in ffnonbonded.itp  :
> > .
> > .
> > .
> > ; Added by DvdS 05/2005 copied from GROMACS force field.
> >  SI         SI     14    28.08000     0.000        A    3.38550e-01
> 2.44704e+00
> >  AU         AU     79   196.9700     0.000       A    0.29510e+00
> 22.1120e+00
> >
> > [ nonbond_params ]
> > AU          AU                                   1    0.00000e+00
> 0.00000e+00
> >
> >
> > ; SC 08/2007: Special Au-N vdw to simulate chemical bond between
> gold-imidazole
> >  AU         opls_511                             1    3.07000e-01
> 3.96000e+00
> >
> > ; SC 05/2008: special Au-C and Au-H to simulate pi-systems
> alkenes+benzene (and PHE)
> >  AU         opls_142                             1    3.21000e-1
> 2.65400e+00
> >  AU         opls_143                             1    3.21000e-1
> 2.65400e+00
> >  AU         opls_144                             1    2.67000e-1
> 1.66500e+00
> >  AU         opls_145                             1    3.20000e-1
> 2.54600e+00
> >  AU         opls_146                             1    2.67000e-1
> 1.66500e+00
> >  AU         opls_150                             1    3.21000e-1
> 2.65400e+00
> >
> > ; +imidazole and His
> >  AU         opls_506                             1    3.21000e-1
> 2.54000e+00
> >  AU         opls_507                             1    3.21000e-1
> 2.54000e+00
> >  AU         opls_508                             1    3.21000e-1
> 2.54000e+00
> >
> > ; +HisH
> >  AU         opls_509                             1    3.21000e-1
> 2.54000e+00
> >  AU         opls_510                             1    3.21000e-1
> 2.54000e+00
> > ; +TYR
> >  AU         opls_166                             1    3.21000e-1
> 2.54000e+00
> > ; +TRP
> >  AU         opls_500                             1    3.21000e-1
> 2.54000e+00
> >  AU         opls_514                             1    3.21000e-1
> 2.54000e+00
> >  AU         opls_501                             1    3.21000e-1
> 2.54000e+00
> >  AU         opls_502                             1    3.55000e-1
> 3.55000e+00
> >
> > and I concidered AU-S as bonding connection and I added its parameter
> (bond stretch, dihedral and angle ) in ffbonded.itp file:
> > [ bondtypes ]
> > ; i    j  func       b0          kb
> > .
> > .
> > .
> > AU    SH      1    0.24000   165528.0   ;
> > AU    S       1    0.24000   165528.0   ;
> > AU    SG      1    0.24000   165528.0   ;
> > .
> > .
> > .
> > [ angletypes ]
> > ;  i    j    k  func       th0       cth
> > .
> > .
> > .
> >   AU     SG     CB      1   109.00     46.34
> >   AU     SH     CB      1   109.00     46.34
> >   AU     S      CB      1   109.00     46.34
> > .
> > .
> > .
> > [ dihedraltypes ]
> > .
> > .
> > .
> > #define improper_AU_S_CB_CA    -180.0      1.2958     2
> >
> > #define improper_AU_SH_CB_CA   -180.0      1.2958     2
> >
> > #define improper_AU_SG_CB_CA    -180       1.2958     2
> >
> > #define improper_AU_S_C_C         19       0.9196     2
> >
> > #define improper_AU_SH_C_C        19       0.9196     2
> >
> > #define improper_AU_SG_C_C        19       0.9196     2
> > .
> > .
> > .
> >
> > when I run my simulation I dont see any interaction or affinity between
> gold atom and S atom of cystein, while it is clear that gold shoud has
> interaction with sulfur. what is its reason? I'm completely confused. I
> tried anythings that I can but my system doesn't work.
> >
> > please help me
> >
> >
> > Fatemeh Ramezani
> > --
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-- 
Cordiali saluti, Dr.Oteri Francesco



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